| Bertrand du Guesclin - Lord of France | Residence at the castle after 1374. |
| Jeanne de Laval - Wife of Du Guesclin | Daughter of Jean de Laval, linked to the castle. |
| André de Laval - Lord of Montsûrs (XIIIth century) | Found four chapelies in the castle. |
| André de Lohéac - Companion of Jeanne d'Arc | Born in the castle of Montsûrs. |
| Comte d'Arundel - Lieutenant-General English | Directed the seat of 1429. |
| Louis XI - King of France | Passed to Montsûrs in 1472. |
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