| Raoul d'Harcourt - Founder of the college (1280) | Chanoine and adviser to Philip IV. |
| Robert d'Harcourt - Bishop of Coutances | Finished the foundation after Raoul's death. |
| Voltaire - Author and former student | First of *The Death of Caesar* in 1735. |
| Jean Racine - Playwright | He studied at Harcourt College. |
| Thomas Fortin - Jansenist Provist (1665–1680) | Close collaborator with Pascal. |
| Jacques Chirac - Former Mayor of Paris | Inaugurated the 700th anniversary plaque (1980). |
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