| Bertrand du Guesclin - Lord and soldier Breton | Residence at the castle after 1374. |
| Jeanne de Laval - Wife of Du Guesclin | Marriage seals the attachment of Laval. |
| André de Lohéac - Companion of Joan of Arc | Born in the enclosure of the castle. |
| Comte d’Arundel - Lieutenant-General English | Ordained destruction in 1429. |
| André de Laval - Lord and Founder | Received Montsûrs in 1292, created chapelies. |
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