| Guérin d'Apchier - Baron d'Acchier | First mention of the castle in 1188. |
| François de Molette - Lord of Morangiès | Transformed the castle in the 17th century. |
| Jean-François-Charles de Molette - Count of Morangiès | Involved in Beast hunting. |
| Frère Hilarion (Joseph-Xavier Tissot) - Religious and doctor | Founded psychiatric asylum in 1824. |
| François Tosquelles - Catalan Psychiatrist | Reformed medical practices in the 20th century. |
| Paul Éluard - Poet resistant | Interned in the castle during the war. |
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